Special Section on Organic Light-Emitting Materials and Devices

Charge-carrier injection and transport in organic light-emitting diodes: Single-particle versus mean-field approach

[+] Author Affiliations
Christian Melzer, Yuri A. Genenko, Sergey V. Yampolskii, Katja Stegmaier, Oliver M. Ottinger, Heinz von Seggern

Technische Universität Darmstadt, Institute of Materials Science, Petersenstrasse 23, Darmstadt, 64287 Germany

J. Photon. Energy. 1(1), 011014 (February 07, 2011). doi:10.1117/1.3534762
History: Received August 12, 2010; Accepted December 15, 2010; Published February 07, 2011; February 10, 2011
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In the framework of the one-dimensional mean-field (MF) drift-diffusion approach the well-defined boundary conditions far away from the metal/insulator contacts of a planar metal/insulator/metal system are used to determine the boundary condition at the interface itself. The novel self-consistent boundary condition linking the carrier density and the electric field at the interface enables a straightforward description of the current voltage (IV) characteristics in forward and reverse bias bridging space charge and injection-limited regimes and accounting for barrier lowering from the potential drop in the used contact materials. Yet, because of the low carrier density in the insulator under injection limitation, single-particle phenomena, such as the Schottky effect, must be considered. We reconsider the validity of the MF approach, depending on the external bias and the prevailing injection barriers. For the crucial parameter window where the MF approach fails and single-particle phenomena become important, a modification of the boundary conditions at the insulator/metal interface is proposed to account for the discrete nature of carriers. The difference between the thus modified MF and the unmodified MF approach is illustrated by several examples.

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© 2011 Society of Photo-Optical Instrumentation Engineers (SPIE)

Citation

Christian Melzer ; Yuri A. Genenko ; Sergey V. Yampolskii ; Katja Stegmaier ; Oliver M. Ottinger, et al.
"Charge-carrier injection and transport in organic light-emitting diodes: Single-particle versus mean-field approach", J. Photon. Energy. 1(1), 011014 (February 07, 2011). ; http://dx.doi.org/10.1117/1.3534762


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