The transport of quantum states without loss of "coherence" is extremely important for realizing quantum information systems. Quantum effects have been demonstrated in exotic systems, such as cold atoms suspended in magnetic fields, but these systems are extremely challenging to realise. In this work we will translate this work into the chemical domain, using thin films of "J-aggregates". These J-aggregates are quantum many-body systems characterized by the sharing of excitonic states over two or more molecules. This novel organic quantum soft-matter platform can confine the light at the nanoscale taking the advantages of supramolecular chemistry to design properties on demand.
Diatoms are an abundant group of algae, sharing a unique feature; they produce silica exoskeletons featuring intricate nanostructures, known as a frustule. In certain species this includes a porous network with high precision lattices, strongly resembling photonic crystals produced using modern technological processes. Here we show two means for using these frustules as an optical material. Firstly, the unprocessed frustule can be used as a conventional photonic crystal. Secondly, a metal deposition processing step can yield plasmonic crystals. Both show high quality optical properties, analogous to lab-manufactured structures, and are produced over much larger areas at a much lower cost and without specialist equipment. Optical spectra (angularly resolved dispersions) are presented, along with simulation results to corroborate experimental findings and to allow optical mode characterisation and analysis.
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