Ultrafast optical control of electron spin is an exciting method for writing magnetic memory with write times on the order of hundreds of femtoseconds. However, most ultrafast optical writing of magnetization has been conducted with high laser fluence (⪆ 1 mJ/cm2) which leads to excessive heating required for deterministic high-power magnetization switching. We present time-resolved magneto-optical Kerr effect observations with laser fluence 1000 times lower than previous studies, to demonstrate low-power optical control of spin in Co/Pd ultrathin multilayers. We observe clear trends between the ferromagnetic layer thickness and significant enhancement in the amplitude of optically excited magnetization precession, and demonstrate the importance of large perpendicular magnetic anisotropy for achieving high sensitivity of electron spin to low power optical excitation. Lastly, we observe a magnetization precession cone angle double of those previously reported which is an important step to achieve a 90-degree precession angle, needed for magnetization switching.
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