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This work is dedicated to laser engineering of spherical resonant Mie-excitonic nanoparticles from layered materials, particularly Transition Metal Dichalcogenides (TMDC). The proposed approach leverages femtosecond laser ablation and fragmentation in liquids for the fabrication of water-dispersed ultra-stable spherical TMDC nanoparticles (NPs) of variable size (5 – 250 nm). Such nanoparticles demonstrate exciting optical and electronic properties inherited from the TMDC crystals, due to preserved crystalline structure, which offers a unique combination of pronounced excitonic response and high refractive index value, making possible a strong concentration of electromagnetic field in nanoparticles.
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Gleb I. Tselikov, Georgy A. Ermolaev, Andrey A. Vyshnevyy, Aleksey V. Arsenin, Valentyn Volkov, "Resonant transition metal dichalcogenide nanoparticles with tunable optical response for nanophotonic applications," Proc. SPIE PC12991, Nanophotonics X, PC129911N (6 June 2024); https://doi.org/10.1117/12.3016390